The effects of viscoelasticity on the dynamics and break-up of fluid threads in microfluidic T-junctions are investigated using numerical simulations of dilute polymer solutions at changing the Capillary number ($\mbox { Ca}$), i.e. at changing the balance between the viscous forces and the surface tension at the interface, up to $\mbox{ Ca} \approx 3 \times 10^{ -2}$. A Navier-Stokes (NS) description of the solvent based on the lattice Boltzmann models (LBM) is here coupled to constitutive equations for finite extensible non-linear elastic dumbbells with the closure proposed by Peterlin (FENE-P model). We present the results of three-dimensional simulations in a range of $\mbox{ Ca}$ which is broad enough to characterize all the three characteristic mechanisms of breakup in the confined T-junction, i.e. ${ \it squeezing}$, ${ \it dripping}$ and ${ \it jetting}$ regimes. The various model parameters of the FENE-P constitutive equations, including the polymer relaxation time $\tau_P$ and the finite extensibility parameter $L^2$, are changed to provide quantitative details on how the dynamics and break-up properties are affected by viscoelasticity. We will analyze cases with ${ \it Droplet ~Viscoelasticity}$ (DV), where viscoelastic properties are confined in the dispersed (d) phase, as well as cases with ${ \it Matrix ~Viscoelasticity}$ (MV), where viscoelastic properties are confined in the continuous (c) phase. Moderate flow-rate ratios $Q \approx { \cal O}(1)$ of the two phases are considered in the present study. Overall, we find that the effects are more pronounced in the case with MV, as the flow driving the break-up process upstream of the emerging thread can be sensibly perturbed by the polymer stresses.

Categories: physics.flu-dyn cond-mat.soft

Effects of viscoelasticity on droplet dynamics and break-up in microfluidic T-Junctions: a lattice Boltzmann study