Exciton, trion and biexciton dephasing rates are measured within the inhomogeneous distribution of an InAs quantum dot (QD) ensemble using two-dimensional Fourier-transform spectroscopy. The dephasing rate of each excitonic state is similar for all QDs in the ensemble and the rates are independent of excitation density. An additional spectral feature -- too weak to be observed in the time-integrated four-wave mixing signal -- appears at high excitation density and is attributed to the $\chi^{ \textrm{ (5)}}$ biexcitonic nonlinear response.

Categories: cond-mat.mes-hall

Fifth-order nonlinear optical response of excitonic states in an InAs quantum dot ensemble measured with 2D spectroscopy